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Low-Temperature Characterization of Domain Wall Dynamics and Electrical Conduction in a Proton-Irradiated K(H$_{0.21}$D$_{0.79}$)$_2$PO$_4$ System

Low-Temperature Characterization of Domain Wall Dynamics and Electrical Conduction in a Proton-Irradiated K(H$_{0.21}$D$_{0.79}$)$_2$PO$_4$ System

초록/요약

We investigated the longitudinal electrical conductivity associated with the domain-wall dynamics in proton-irradiated K(H$_{0.21}$D$_{0.79}$)$_2$PO$_4$ single crystals a temperatures below room temperature. Frequency-dependent longitudinal dielectric-loss measurements allowed us to investigate the changes in the domain-wall dynamics of the proton-irradiated crystal with a ferroelectric phase-transition temperature increase of 8 K. Using the Vogel-Fulcher function, we found that proton irradiation produced a slight increase in the activation energy of domain freezing. The temperature dependence of the power-law exponent $n$ in frequency-dependent electrical conductivity in proton-conducting systems decreased at temperatures near the phase-transition temperature $T_{c2}$. In addition, the temperature dependence of the electrical conductivity shifted to higher temperatures because of the increased phase-transition temperature arising from the proton irradiation.

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